[1]袁柯馨,孙荣,李玉,等.城市污泥中重金属形态及资源化可行性分析[J].华侨大学学报(自然科学版),2014,35(4):424-429.[doi:10.11830/ISSN.1000-5013.2014.04.0]
 YUAN Ke-xin,SUN Rong,LI Yu,et al.Form of Heavy Metals in Sewage Sludge and Resource Feasibility in Southern City[J].Journal of Huaqiao University(Natural Science),2014,35(4):424-429.[doi:10.11830/ISSN.1000-5013.2014.04.0]
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城市污泥中重金属形态及资源化可行性分析()
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《华侨大学学报(自然科学版)》[ISSN:1000-5013/CN:35-1079/N]

卷:
第35卷
期数:
2014年第4期
页码:
424-429
栏目:
出版日期:
2014-07-10

文章信息/Info

Title:
Form of Heavy Metals in Sewage Sludge and Resource Feasibility in Southern City
文章编号:
1000-5013(2014)04-0424-06
作者:
袁柯馨 孙荣 李玉 洪俊明
华侨大学 化工学院, 福建 厦门 361021
Author(s):
YUAN Ke-xin SUN Rong LI Yu HONG Jun-ming
College of Chemical Engineering, Huaqiao University, Xiamen 361021, China
关键词:
污泥 重金属 形态分布 资源化
Keywords:
sewage sludge heavy metal form distribution resource
分类号:
X703
DOI:
10.11830/ISSN.1000-5013.2014.04.0
文献标志码:
A
摘要:
以南方某市6个污水处理厂为例,分析污泥中重金属Cu,Zn,Ni,Pb,Cd,Cr的质量比及其形态分布特征,分析污泥农用的最大施用量和制砖的最大添加量.结果表明:污泥中的Pb,Ni,Cd有效态比例较高,Zn,Cr主要以不可利用态存在,Cu主要以潜在有效态和不可利用态存在.污泥农用的静态环境容量分析结果显示:不同来源污泥的最大施用量有显著差异,可将Cd作为主要监控污染元素,同时作为控制城市污水污泥农用过程中最高施用量的计算参考指标,以保证土壤环境安全.通过制砖污泥添加比例的计算,选取Cu作为E污水厂污泥制砖过程的限制性指标,其余5个污水处理厂的限制性指标为Cr.
Abstract:
The content and form distribution of heavy metals(Cu, Zn, Ni, Pb, Cd, Cr)from sewage sludge in six wastewater treatment plants in a southern city of China were investigated. The maximum amount of sewage sludge which could be applied to agricultural soil and brick was also calculated. Results revealed that Zn and Cr existed mainly in unavailable form, and Cu was in a state of potentially effective and unavailable fraction. The effective proportions of Pb, Ni and Cd were larger than other metals. As calculated by the static environmental capacity of latosolic red solid of the city, the main detected harmful heavy metal was Cd in the course of agriculture utilization of sludge. The maximum application amount of sludge from various sources were significantly different. Therefore, we suggested that the content of Cd in sewage sludge could be used as a reference index, which was used for calculating the maximal application rate in the control of application rate of sludge for agricultural land, and for the protection of solid environment. As calculated by the addition ratio of the sewage sludge in the brick, the main control index was Cu in the E wastewater treatment plant, meanwhile Cr was selected as the dangerous heavy metal in the other five wastewater treatment plants.

参考文献/References:

[1] 杨军,郭广慧,陈同斌,等.中国城市污泥的重金属含量及其变化趋势[J].中国给水排水,2009,25(13):122-124.
[2] FYTILI D,ZABANIOTOU A.Utilization of sewage sludge in EU application of old and new method: A review[J].Renewable and Sustainable Energy Reviews,2008,12(1):116-140.
[3] 胡绵好,袁菊红,黄和平,等.南昌市城市污泥重金属形态分布及其生物活性研究[J].水土保持通报,2010,30(5):64-67.
[4] BASEM S I K,KALAVROUZIOTIS P H,KOUKOULAKIS A Y.Soil pollution indices under the effect of sludge[J].Water, Air and Soil Pollution,2013,224(2):1436-1441.
[5] IMPELLITTERI C A,SAXE J K,COCHRAN M,et al.Predicting the bioavailability of copper and zinc in soils: Modeling the partitioning of potentially bioavailable copper and zinc from soil solid to soil solution[J].Environmental Toxicology and Chemistry,2003,22(6):1380-1386.
[6] SASTRE J,HERNANDEZ E,RODRIGUEZ R,et al.Use of sorption and extraction tests to predict the dynamics of the interaction of trace elements in agricultural soils contaminated by a mine tailing accident[J].Science of the Total Environment,2004,329(1/2/3):261-281.
[7] 谢莹,张涛,金建峰,等.污水处理厂脱水污泥中重金属的形态分布特征研究[J].中国给水排水,2012,28(5):93-96.
[8] 姚金铃,王海燕,于云江,等.城市污水处理厂污泥重金属污染状况及特征[J].环境科学研究,2010,23(6):676-702.
[9] 张丽丽,李花粉,苏德纯.我国城市污水处理厂污泥中重金属分布特征及变化规律[J].环境科学研究,2013,26(3):313-319.
[10] TESSIER A,CAMPBELL P G C,BISSON M.Sequential extraction procedure for the speciation of particulate trace metals[J].Analytical Chemistry,1979,51(7):844-851.
[11] 邱海源.厦门市翔安区土壤重金属分布、形态及生态效应研究[D].厦门:厦门大学,2008:163-165.
[12] 于瑞莲,胡恭任,张丽玲.泉州城市污泥中重金属赋存形态和生物有效性分析[J].环境化学,2011,30(11):1965-1966.
[13] 姜勇,梁文举,张玉革,等.污灌对土壤重金属环境容量及水稻生长的影响研究[J].中国生态农业学报,2004,12(3):124-127.
[14] 冯春,杨光,杜俊,等.污水污泥堆肥重金属总量及形态变化[J].环境科学研究,2008,21(1):97-102.
[15] 李淑更,张可方,周少奇,等.脱水污泥在美人蕉种植中的应用[J].环境科学研究,2008,21(2):158-162.
[16] 马雯,呼世斌.以城市污泥为掺量制备烧结砖[J].环境工程学报,2012,6(3):1035-1038.
[17] OBRADOR A,RICO M I,ALVAREZ J M,et al.Influence of thermal treatment on sequential extraction and leaching behavior of trace metals in a contaminated sewage sludge[J].Bioresource Technology,2001,76(3):259-264.

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备注/Memo

备注/Memo:
收稿日期: 2013-09-04
通信作者: 洪俊明(1974-),男,副教授,主要从事水污染控制工程及清洁生产的研究.E-mail:jmhong@hqu.edu.cn.
基金项目: 国家水专项城市污水处理系统运行特性与工艺设计技术研究项目(2012ZX07313-001); 福建省厦门市科技计划项目(3502Z20110008, 3502Z20123029)
更新日期/Last Update: 2014-07-20