[1]谢艳梅,吴季怀,林建明,等.铬掺杂钙铌酸的制备及其光催化性能[J].华侨大学学报(自然科学版),2008,29(2):256-259.[doi:10.11830/ISSN.1000-5013.2008.02.0256]
 XIE Yan-mei,WU Ji-huai,LIN Jian-ming,et al.Synthesis and Photochemical Properties of Cr-Doped HCa2Nb3O10[J].Journal of Huaqiao University(Natural Science),2008,29(2):256-259.[doi:10.11830/ISSN.1000-5013.2008.02.0256]
点击复制

铬掺杂钙铌酸的制备及其光催化性能()
分享到:

《华侨大学学报(自然科学版)》[ISSN:1000-5013/CN:35-1079/N]

卷:
第29卷
期数:
2008年第2期
页码:
256-259
栏目:
出版日期:
2008-04-20

文章信息/Info

Title:
Synthesis and Photochemical Properties of Cr-Doped HCa2Nb3O10
文章编号:
1000-5013(2008)02-0256-04
作者:
谢艳梅吴季怀林建明黄妙良黄昀昉
华侨大学材料科学与工程学院; 华侨大学材料科学与工程学院 福建泉州362021; 福建泉州362021
Author(s):
XIE Yan-mei WU Ji-huai LIN Jian-ming HUANG Miao-liang HUANG Yun-fang
College of Material Science and Engineering, Huaqiao University, Quanzhou 362021, China
关键词:
HCa2Nb3O10 光催化 掺杂 氢气
Keywords:
HCa2Nb3O10 chromium photocatalysis doping hydrogen
分类号:
O614.3
DOI:
10.11830/ISSN.1000-5013.2008.02.0256
文献标志码:
A
摘要:
通过高温固相反应制备铬掺杂的钙铌酸钾系列样品,并用离子交换反应制备出对应的铬掺杂钙铌酸样品.采用X-射线衍射、紫外-可见漫反射光谱、扫描电镜等方法,对所制得的样品进行表征.在甲醇为电子给体,Pt为助催化剂的情况下,研究铬掺杂的钙铌酸系列催化剂,在波长大于290 nm紫外光辐射下分解水产氢的光催化活性.结果表明,适量的掺杂铬可有效地提高钙铌酸的光催化分解水的活性.最后,讨论引起催化剂活性差异的可能原因.
Abstract:
The photocatalysts series HCa2Nb3O10 doped with Cr3+ were prepared by conventional solid-state reactions followed by an ion-exchange reaction.The samples were characterized by powder X-ray diffraction,UV-Vis diffusive reflectance spectrum and scanning electron microscope.The photocatalytic activities of HCa2Nb3O10 doped with Cr3+are investigated with methanol as electron donor and Pt as promoter catalyst under irradiation of UV light with wavelength more than 290 nm.The results show that the doping of Cr3+ improves the photocatalytic activity of HCa2Nb3O10,the difference of photocatalytic activity among them is also discussed.

参考文献/References:

[1] FJISHIMA A, HONDA K. Electrochemical photolysis of water at a semiconductor electrode [J]. Nature, 1972, (5358):37-38.
[2] THAMINIMULLA C T K, TAKATA T, HARA M. Effect of chromium addition for photocatalytic overall water splitting on Ni-K2La2Ti3O10 [J]. Journal of Catalysis, 2000, (2):362-365.doi:10.1006/jcat.2000.3049.
[3] WU Ji-huai, UCHIDA S, FUJISHIRO Y. Synthesis and photocatalytic properties of HNbWO6/TiO2 and of HNbWO6/Fe2O3 nanocompsites [J]. Journal of Photochemistry and Photobiology A:Chemistry, 1999, (11):129-133.
[4] YANAGISAWA M, UCHIDA S, SATO T. Synthesis and photochemical properties of Cu2+ doped layered hydrogen titanate [J]. International Journal of Inorganic Materials, 2000(2):339-346.doi:10.1016/S1466-6049(00)00033-7.
[5] HWANG D W, KIM H G, KIM J. Photocatalytic water splitting over highly donor-doped (110) layered perovskites [J]. Journal of Catalysis, 2000, (1):40-48.doi:10.1006/jcat.2000.2875.
[6] KUDO A, KATO H. Effect of lanthanide-doping into NaTaO3 photcatalysts for efficient water splitting [J]. Chemical Physics Letters, 2000, (331):373-377.doi:10.1016/S0009-2614(00)01220-3.
[7] SATO T, FUKUGAMI Y. Synthesis and photocatalytic properties of TiO2 and Pt pillared HCa2Nb3O10 doped with various rare earth ions [J]. Solid-State Ionicis, 2001, (141-142):397-405.doi:10.1016/S0167-2738(01)00804-9.
[8] ZOU Zhi-gang, YE Jin-hua, SAYAMA K. Photocatalytic and photophysical properties of a novel series of solid photocatalysts, BiTa1-xNbxO4(0≤x≤1) [J]. Chemical Physics Letters, 2001.303-308.
[9] ZOU Zhi-gang, YE Jin-hua, KAZUHIRO S, HIRONORI A. Photocatalytic hydrogen and oxygen formation under visible light irradiation with M-doped InTaO4(M=Mn, Fe, Co, Ni and Cu) photocatalysts [J]. Journal of Photochemistry and Photobiology A:Chemistry, 2002.65-69.doi:10.1016/S1010-6030(02)00068-0.
[10] 陈建华, 王晓林, 龚竹青. Cr3+掺杂对TiO2薄膜光催化活性的影响 [J]. 环境科学学报, 2005(5):606-610.doi:10.3321/j.issn:0253-2468.2005.05.007.
[11] 杨亚辉, 陈启元, 尹周澜. Fe3+ 和Cr3+ 掺杂对K4Nb6O17光催化活性的影响 [J]. 中国稀土学报, 2004(5):647-650.doi:10.3321/j.issn:1000-4343.2004.05.013.
[12] 傅希贤, 杨秋华, 桑丽霞. 钙钛矿型LaFe1-xCuxO3的光催化活性研究 [J]. 高等学校化学学报, 2002(2):283-286.doi:10.3321/j.issn:0251-0790.2002.02.020.
[13] ZOU Zhi-gang, YE Jin-hua, SAYAMA K. Direct splitting of water under visible light irradiation with an oxide semiconductor photocatalyst [J]. Nature, 2001.625-627.
[14] 傅希贤, 桑丽霞, 白树林. LaFe1-xCuxO3的光催化性能及正电子湮没研究 [J]. 化学物理学报, 2000(4):503-507.doi:10.3969/j.issn.1674-0068.2000.04.019.

相似文献/References:

[1]林碧洲.某些有机铵十聚钨酸盐的制备和催化性质[J].华侨大学学报(自然科学版),2002,23(3):300.[doi:10.3969/j.issn.1000-5013.2002.03.017]
 Lin Bizhou.Preparation and Catalytic Properties of Some Organoammonium Decatungstates[J].Journal of Huaqiao University(Natural Science),2002,23(2):300.[doi:10.3969/j.issn.1000-5013.2002.03.017]
[2]刘如东,薛秀玲.纳米TiO2-xNx光催化薄膜的制备及其性能表征[J].华侨大学学报(自然科学版),2010,31(4):438.[doi:10.11830/ISSN.1000-5013.2010.04.0438]
 LIU Ru-dong,XUE Xiu-ling.Preparation and Characterization of Nitrogen-Doped Nano-TiO2 Photocatalytic Film[J].Journal of Huaqiao University(Natural Science),2010,31(2):438.[doi:10.11830/ISSN.1000-5013.2010.04.0438]
[3]陈亦琳,陈林峰.Ag2O光催化过程中单质Ag的生成及作用机理[J].华侨大学学报(自然科学版),2011,32(6):652.[doi:10.11830/ISSN.1000-5013.2011.06.0652]
 CHEN Yi-lin,CHEN Lin-feng.Study on Effect and Mechanism of Metallic Ag in the Photocatalytic Process by Ag2O[J].Journal of Huaqiao University(Natural Science),2011,32(2):652.[doi:10.11830/ISSN.1000-5013.2011.06.0652]
[4]陈晶玲,兰心仁,金春英.表面键合型CO2-3/TiO2光催化剂的性能表征[J].华侨大学学报(自然科学版),2013,34(5):534.[doi:10.11830/ISSN.1000-5013.2013.05.0534]
 CHEN Jing-ling,LAN Xin-ren,JIN Chun-ying.Performance Characterization of Surface CO2-3-Bonded TiO2 Photocatalyst[J].Journal of Huaqiao University(Natural Science),2013,34(2):534.[doi:10.11830/ISSN.1000-5013.2013.05.0534]

备注/Memo

备注/Memo:
国家自然科学基金资助项目(50572030,50372022)
更新日期/Last Update: 2014-03-23